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固体氧化物燃料电池 8

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Latest development of double perovskite electrode materials for solid oxide fuel cells: a review

Shammya AFROZE, AfizulHakem KARIM, Quentin CHEOK, Sten ERIKSSON, Abul K. AZAD

《能源前沿（英文）》 2019年第13卷第4期页码 770-797 doi: 10.1007/s11708-019-0651-x

摘要： Recently, the development and fabrication of electrode component of the solid oxide fuel cell (SOFC) have gained a significant importance, especially after the advent of electrode supported SOFCs. The function of the electrode involves the facilitation of fuel gas diffusion, oxidation of the fuel, transport of electrons, and transport of the byproduct of the electrochemical reaction. Impressive progress has been made in the development of alternative electrode materials with mixed conducting properties and a few of the other composite cermets. During the operation of a SOFC, it is necessary to avoid carburization and sulfidation problems. The present review focuses on the various aspects pertaining to a potential electrode material, the double perovskite, as an anode and cathode in the SOFC. More than 150 SOFCs electrode compositions which had been investigated in the literature have been analyzed. An evaluation has been performed in terms of phase, structure, diffraction pattern, electrical conductivity, and power density. Various methods adopted to determine the quality of electrode component have been provided in detail. This review comprises the literature values to suggest possible direction for future research.

关键词： double perovskites electrode materials hydrocarbon fuel solid oxide fuel cells

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Emission components characteristics of a bi-fuel vehicle at idling condition

Sameh M. METWALLEY, Shawki A. ABOUEL-SEOUD, Abdelfattah M. FARAHAT

《能源前沿（英文）》 2011年第5卷第3期页码 322-329 doi: 10.1007/s11708-011-0158-6

摘要： Natural gas (NG) represents today a promising alternative to conventional fuels for road vehicles propulsion, since it is characterized by a relatively low cost, better geopolitical distribution than oil, and lower environmental impact. This explains the current spreading of compressed natural gas (CNG) fuelled spark ignition (SI) engine, above all in the bi-fuel version, which is able to run either with gasoline or with NG. However, the aim of the present investigation is to evaluate the emission characteristics at idling condition. The vehicle engine was converted to bi-fueling system from a gasoline engine, and operated separately either with gasoline or CNG. Two different fuel injection systems (i.e., multi-point injection (MPI)-sequential and closed-loop venturi-continuous) are used, and their influences on the formation of emissions at different operating conditions are examined. A detailed comparative analysis of the engine exhaust emissions using gasoline and CNG is made. The results indicate that the CNG shows low air index and lower emissions of carbon monoxide (CO), carbon dioxide (CO ), and total hydrocarbon (THC) compared to gasoline.

关键词： road vehicle engine fuel injection systems carbon monoxide (CO) carbon dioxide (CO₂) total hydrocarbon (THC) vehicle idle conditions air index

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中国古生代海相油气成藏特征

康玉柱

《中国工程科学》 2010年第12卷第5期页码 11-17

摘要：

1970―1978年笔者在塔里木油气地质调研中首次提出古生代有发育的烃源岩，1984年沙参2井实现了古生代海相油田的首次重大突破。1992年通过多个古生代油气田深入研究建立了古生代海相油气成藏理论。其理论内涵：叠加复合盆地成藏，多时代多层系生油，多期成藏，多时代多类型储盖组合，多成藏模式，油气主要分布在古隆起、古斜坡、断裂带和不整合面附近。

关键词：古生代海相油气田盆地隆起坳陷油气分布

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exogenous degrader-enhanced bioremediation with low-dose persulfate oxidation for polycyclic aromatic hydrocarbon

《环境科学与工程前沿（英文）》 2023年第17卷第11期 doi: 10.1007/s11783-023-1733-x

摘要： Polycyclic aromatic hydrocarbon (PAH)-contaminated soils are usually complex and characterized by a lack of nutrition and soil salinization, resulting in difficulties in soil remediation. In this study, bioaugmentation with a PAH-degrading Bacillus PheN7 (BA) and low-dose persulfate oxidation (PS), along with natural biodegradation, were utilized to remediate alkaline PAH-contaminated soil. The soil used in the study had a pH of 9.35, and the total PAH content was 568.8 ± 31.0 mg/kg dry soil. After 42 d of remediation, the degradation efficiency of PAHs was 96.72% and 93.88% using persulfate oxidation and bioaugmentation, respectively, whereas 38.66% of PAHs were degraded in natural attenuation (NA). Bacillus was the dominant genera throughout the process of bioremediation with the relative abundance of 79.3% on day 42 in the BA system, whereas, Alcanivorax was enriched and became the dominant genera in PS systems. In the meantime, PAH degradation genes were detected with remarkably higher level in the BA system than in PS system during the remediation. In addition to the degradation of contaminants, persulfate oxidation promotes microbial bioremediation efficiency mainly by lowering the pH to neutral and increasing the active phosphorus content in the soil. Microbial species and ecological niches were less reduced in the PS system than in the BA system. Collectively, persulfate oxidation had a better impact on the soil microbiome and is more suitable for long-term soil health than bioaugmentation through PheN7 addition.

关键词： Bioaugmentation Low-dose persulfate oxidation Polycyclic aromatic hydrocarbon Remediation

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中国非常规油气的潜力和发展

胡文瑞,翟光明,李景明

《中国工程科学》 2010年第12卷第5期页码 25-29

摘要：

概述了国外和我国非常规油气资源开发利用状况，分析了我国发展非常规油气存在的困难，提出了加快发展我国非常规油气的对策与建议。

关键词：非常规油气勘探开发技术潜力对策

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中国石化非常规油气资源潜力及勘探进展

马永生,冯建辉,牟泽辉,赵培荣,包书景,王烽

《中国工程科学》 2012年第14卷第6期页码 22-30

摘要：

中国石油化工集团有限公司（简称中国石化）矿权区内拥有较为丰富的非常规油气资源，煤层气可勘探面积为10.19万km²，煤层埋深小于2 000 m的煤层气地质资源量为11.02万亿m³。页岩气可供勘探面积为17.5万km²，初步估算页岩气地质资源量为15.9万亿m³。页岩油勘探面积为11.76万km²，具有较大的资源基础及潜力。中国石化自2004年开始关注非常规油气资源，先后启动了页岩油气、煤层气等非常规油气资源的研究和勘探工作。目前在泌阳凹陷页岩油勘探泌页HF-1水平井分段压裂后获日产油23.6 m³；元坝地区多口陆相钻井测试获得高产气流，建南地区建页HF-1井日产气12 300 m³；延川南区块煤层气已探明地质储量为106.47亿m³，多口井排采获工业气流，初步形成了中国石化非常规油气资源多类型、多阶段的勘探开发格局。

关键词：中国石化非常规油气油气资源勘探

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轻烃分析录井技术在海拉尔盆地的应用

吴长金,马昌伟,张可操

《中国工程科学》 2012年第14卷第4期页码 49-57

摘要：

为适应海拉尔盆地快速勘探开发工作的需要，有效解决在快速钻井（钻井提速）条件下，岩屑录井、地化录井等依托岩屑样品发现油气显示以及评价储层所面临的技术难题，按照优选先进适用录井技术的要求，在海拉尔盆地进行了轻烃分析录井技术应用。笔者阐述了轻烃分析录井技术的原理和特点，并对该项技术的实际应用效果进行了分析，为轻烃分析录井技术的推广应用奠定了坚实基础。

关键词：海拉尔盆地轻烃分析录井技术油气发现储层评价

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Deepwater Hydrocarbon Exploration in China Seas: Yesterday, Today and Tomorrow

Zhi-gang Zhao,Hai-zhang Yang,Wu Tang,Shi-xiang Liu

《工程管理前沿（英文）》 2016年第3卷第4期页码 390-395 doi: 10.15302/J-FEM-2016059

摘要： Deepwater area has been one of the hottest areas in the global hydrocarbon exploration. However, deepwater hydrocarbon exploration in China started late and mainly concentrated in the South China Sea (SCS) with low level of researches. Although there are some achievements, there are even more challenges. For this reason, this paper reviewed the history of deepwater exploration in China Seas and summarized the current exploration situation. The future directions of deepwater hydrocarbon exploration mainly consist of five aspects: establishing key technology system of complex structure and reservoir seismic acquisition and processing in deepwater areas of SCS, clarifying the development mechanism of high quality source rock and establishing matching assessment technology, studying the formation conditions of favorable reservoir and creating reservoir identification technology, improving accumulation theory of large and medium-sized oil and gas field of deepwater, deepening the researches of petroleum geology conditions of middle and south part of SCS. Simultaneously, the concept of portfolio should be utilized in the exploration process, with economic benefits considered. These understandings will help guiding the future deepwater hydrocarbon exploration in China Seas.

关键词： deepwater hydrocarbon exploration China Seas South China Sea Pearl River Mouth Basin Qiongdongnan Basin development directions

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碳基固体氧化物燃料电池理论模拟概述

李家玉,王宝轩,陈美娜,李昂,方秀荣,宋策,林子敬

《中国工程科学》 2013年第15卷第2期页码 39-49

摘要：

主要对碳基固体氧化物燃料电池（SOFC）中三传二反的控制方程、不同尺度的不同物理场理论模型以及碳基燃料的重整、催化和硫化等方面进行概括总结。SOFC有可使用氢气、一氧化碳、甲烷和其他的碳氢化合物作为燃料进行电化学反应的燃料灵活性，但使用碳氢燃料需要解决诸如碳基燃料的重整、电极的催化、积碳和硫化等问题。电池内部反应气体的物质输运、电荷输运、能量输运、动量输运和化学及电化学反应状态均可以用偏微分方程来描述。运用这些电化学反应和输运的偏微分方程，结合材料的微观性质，可以建立SOFC的多尺度多物理场模型。通过理论模型研究材料微结构与性质、工作条件、几何构型等参数对电池性能的影响，对SOFC材料组成与电池堆结构进行定量分析和优化设计，可以加速SOFC技术的更快发展。

关键词：多尺度模拟结构性能优化重整反应催化硫化

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Reduced kinetic mechanism of -heptane oxidation in modeling polycyclic aromatic hydrocarbon formation

ZHONG Beijing, XI Jun

《能源前沿（英文）》 2008年第2卷第3期页码 326-332 doi: 10.1007/s11708-008-0047-9

摘要： A reduced mechanism, which could couple with the multidimensional computational fluid dynamics code for quantitative description of a reacting flow, was developed for chemical kinetic modeling of polycyclic aromatic hydrocarbon formation in an opposed-flow diffusion flame. The complete kinetic mechanism, which comprises 572 reactions and 108 species, was reduced to a simplified mechanism that includes only 83 reactions and 56 species through sensitivity analysis. The results computed via this reduced mechanism are nearly indistinguishable from those via the detailed mechanism, which demonstrate that the model based on this reduced mechanism can properly describe -heptane oxidation chemistry and quantitatively predict polycyclic aromatic hydrocarbon (such as benzene, naphthalene, phenanthrene and pyrene) formation in opposed-flow diffusion flames.

关键词： phenanthrene multidimensional computational sensitivity analysis polycyclic mechanism

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Combustion and emissions of RP-3 jet fuel and diesel fuel in a single-cylinder diesel engine

《能源前沿（英文）》 2023年第17卷第5期页码 664-677 doi: 10.1007/s11708-021-0787-3

摘要： The combustion characteristics and emission behaviors of RP-3 jet fuel were studied and compared to commercial diesel fuel in a single-cylinder compression ignition (CI) engine. Engine operational parameters, including engine load (0.6, 0.7, and 0.8 MPa indicating the mean effective pressure (IMEP)), the exhaust gas recirculation (EGR) rate (0%, 10%, 20%, and 30%), and the fuel injection timing (−20, −15, −10, and −5 ° crank angle (CA) after top dead center (ATDC)) were adjusted to evaluate the engine performances of RP-3 jet fuel under changed operation conditions. In comparison to diesel fuel, RP-3 jet fuel shows a retarded heat release and lagged combustion phase, which is more obvious under heavy EGR rate conditions. In addition, the higher premixed combustion fraction of RP-3 jet fuel leads to a higher first-stage heat release peak than diesel fuel under all testing conditions. As a result, RP-3 jet fuel features a longer ignition delay (ID) time, a shorter combustion duration (CD), and an earlier CA50 than diesel fuel. The experimental results manifest that RP-3 jet fuel has a slightly lower indicated thermal efficiency (ITE) compared to diesel fuel, but the ITE difference becomes less noticeable under large EGR rate conditions. Compared with diesel fuel, the nitrogen oxides (NO_x) emissions of RP-3 jet fuel are higher while its soot emissions are lower. The NO_x emissions of RP-3 can be effectively reduced with the increased EGR rate and delayed injection timing.

关键词： RP-3 jet fuel diesel engine combustion emissions

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Impacts of methanol fuel on vehicular emissions: A review

《环境科学与工程前沿（英文）》 2022年第16卷第9期 doi: 10.1007/s11783-022-1553-4

摘要：

● Methanol effectively reduces CO, HC, CO₂, PM, and PN emissions of gasoline vehicles.

关键词： Methanol fuel Vehicular emission Emission reduction Cleaner fuel Gasoline substitute

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地下水封岩洞油库设计、施工的基本原则

王梦恕,杨会军

《中国工程科学》 2008年第10卷第4期页码 11-16

摘要：

我国对大量石油储存的需求使石油贮备库的建设势在必行，地下水封岩洞油库是储存油品的最好形式。文章介绍了地下水封岩洞油库的密封原理、类型、优点等并重点对其选址、设计、施工进行介绍。笔者旨在提出地下水封岩洞油库的主要特点和规划、设计、施工的基本原则及标准，并指出我国尚未形成关于大规模地下水封岩洞油库设计、施工的完整技术，缺少指导性规范。开展地下水封岩洞油库的关键设计与施工技术研究具有重大的现实意义。

关键词：地下水封储油库岩洞设计施工

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Failure mode investigation of fuel cell for vehicle application

Zhongjun HOU, Renfang WANG, Keyong WANG, Weiyu SHI, Danming XING, Hongchun JIANG

《能源前沿（英文）》 2017年第11卷第3期页码 318-325 doi: 10.1007/s11708-017-0488-0

摘要： The durability of proton exchange membrane fuel cells (PEMFCs) has been posing a key technical challenge to commercial spread of fuel cell vehicles (FCVs). To improve the durability, it is necessary to optimize the fuel cell system (FCS) design against failure modes. The fuel cell durability research method at FCS scale was exhibited, and the failure modes of fuel cell were experimentally investigated in this paper. It is found that the fuel cell dry operation, start/stop cycle and gas diffusion layer (GDL) flooding are typical failure modes of fuel cells. After the modifications against the failure modes, the durability of FCSs is improved to over 3000 h step by step.

关键词： proton exchange membrane fuel cell (PEMFC) fuel cell system (FCS) durability failure mode fuel cell vehicle (FCV) carbon corrosion water management

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Numerical investigation of the effects of fuel spray type on the interaction of fuel spray and hot porous

ZHAO Zhiguo, XIE Maozhao

《能源前沿（英文）》 2008年第2卷第1期页码 59-65 doi: 10.1007/s11708-008-0022-5

摘要： The interaction between two types of fuel spray and a hot porous medium is studied numerically by using an improved version of KIVA-3V code. The improved KIVA-3V code is incorporated with an impingement model, a heat transfer model and a linearized instability sheet atomization (LISA) model to model the hollow cone spray. An evaporating fuel spray impingement on a hot plane surface was simulated under conditions of experiments performed by Senda to validate the reasonability of the KIVA-3V code. The numerical results conform well with experimental data for spray radius in the liquid and the vapor phases. Computational results on the interaction of two types of the fuel spray and the hot porous medium show that the fuel spray can be split, which provides conditions for quick evaporation of fuel droplets and mixing of fuel vapor with air. The possibility of fuel droplets from hollow cone spray crossing the porous medium reduces compared with that from solid cone spray, with the same initial kinetic energy of fuel droplets in both injection types.

关键词： improved version impingement atomization hollow radius